刘平副教授、孙培培教授课题组在ORGANIC LETTERS发表研究论文

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Selective C-5 Oxidative Radical Silylation of Imidazopyridines Promoted by Lewis Acid
Li, YF (Li, Yifan)[ 1 ] ; Shu, KC (Shu, Kaichen)[ 1 ] ; Liu, P (Liu, Ping)[ 1 ]*(刘平); Sun, PP (Sun, Peipei)[ 1 ]*(孙培培)

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[ 1 ] Nanjing Normal Univ, Jiangsu Collaborat Innovat Ctr Biomed Funct Mat, Sch Chem & Mat Sci, Jiangsu Prov Key Lab Mat Cycle Proc & Pollut Cont, Nanjing 210023, Peoples R China

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亚博app买球首选:ORGANIC LETTERS,202008,22(16),6304-6307

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An oxidative cross dehydrogenative coupling of imidazopyridines with silanes was developed using di-tert-butyl peroxide as the oxidant. The coordination effect of Lewis acid was the dominant factor controlling the regioselective addition of silyl radical to imidazopyridines, and the corresponding C-5 silylated imidazo[1,2-a]pyridines were obtained in moderate to high yields with a broad substrate scope.

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